/Dicke State and Holstein–Primakoff transformation

Dicke State and Holstein–Primakoff transformation

Sections13
  1. Collective spin operators
  2. Define
  3. Commutation
  4. Effective z-value component spin
  5. Dicke state Basis
  6. Raising and Lowering
  7. Holstein–Primakoff Transformation
  8. Weak Excitation Regime
  9. Beam splitter
  10. Collective Rabi Oscillations and Quantum Memory
  11. Superradiance and Subradiance from Decay Rates
  12. Superradiance and the Superradiant Burst
  13. Subradiance

Collective spin operators§

Define§

S^±=∑iσ^(i)±S^e=∑iσ^e(i)S^g=∑iσ^g(i)S^z=12∑iσ^z(i)\hat S_\pm = \sum_i{\hat\sigma_{(i)}^\pm} \qquad \hat S_e=\sum_i{\hat\sigma_e^{(i)}}\qquad \hat S_g=\sum_i{\hat\sigma_g^{(i)}} \qquad \hat S_z=\frac{1}{2}\sum_i{\hat\sigma_z^{(i)}}

Commutation§

With linearity of commutator, easily we see that this definition of collective spin makes sense, and also obeys the single atom spin commutation relation.

[S^+,S^−]=2S^zetc...\left[\hat S_+, \hat S_-\right]=2\hat S_z \qquad \text{etc...}

Effective z-value component spin§

Just as single atom spin could have a z-component, here, easily we note that from

Sz=12∑iσ^z(i)=∑iσ^e(i)−N2S_z=\frac{1}{2}\sum_i{\hat\sigma_z^{(i)}} = \sum_{i}\hat\sigma_e^{(i)}-\frac{N}{2}

z-component will be in {N/2,N/2−1,…,−N/2}\{N/2, N/2 - 1, \dots,-N/2\}, call this mm

Dicke state Basis§

So, sufficiently by SS and mm (assuming all states act coherently), we define a basis

∣S,m⟩=1(Nne)∑perm∣eee…⏟neggg…⏟ng⟩\ket{S,m}=\frac{1}{\sqrt{\binom{N}{n_e}}}\sum_{\text{perm}}\ket{\underbrace{eee\dots}_{n_e} \underbrace{ggg\dots}_{n_g}}

Where ne=S+mn_e=S+m, ng=S−mn_g=S-m

Raising and Lowering§

S^−∣S,m⟩=S(S+1)−m(m−1)∣S,m−1⟩S^+∣S,m⟩=S(S+1)−m(m+1)∣S,m+1⟩\hat S_-\ket{S,m}=\sqrt{S(S+1)-m(m-1)}\ket{S,m-1}\qquad \hat S_+\ket{S,m}=\sqrt{S(S+1)-m(m+1)}\ket{S,m+1}

For large enough NN,

S2−m2+S+m=(S+m)(S−m+1)=ne(ng+1)\sqrt{S^2-m^2+S+m}=\sqrt{(S+m)(S-m+1)}=\sqrt{n_e(n_g+1)} S2−m2+S−m=(S+m+1)(S−m)=(ne+1)ng≈neng\sqrt{S^2-m^2+S-m}=\sqrt{(S+m+1)(S-m)}=\sqrt{(n_e+1)n_g}\approx\sqrt{n_en_g}

Thus, ⟨S^+S^−⟩=ne(ng+1)\braket{\hat S^+\hat S^-}=n_e(n_g+1). The point here is the coherence of the Dicke-state depends on both nen_e and ngn_g, differing from the expectation if all atoms go out of phase.

Holstein–Primakoff Transformation§

We aim to treat this ensemble as a single bosonic wave when interacting with a single photon, or at least approximately. Doing so provides practical use for the formalism developed above.

Thus, we take the ansatz. We want

S^z=c^†c^−N2S^+=c^†N−c^†c^S−=N−c^†c^ c^[c^,c^†]=1\hat S_z = \hat c^\dagger \hat c - \frac{N}{2}\qquad \hat S_+ = \hat c^\dagger \sqrt{N-\hat c^\dagger \hat c} \qquad S_- = \sqrt{N-\hat c^\dagger \hat c}\,\hat c\qquad [\hat c,\hat c^\dagger]=1

Then, we will have

[S^+,S^−]=2S^zetc...\left[\hat S_+, \hat S_-\right]=2\hat S_z \qquad \text{etc...}

And if c^†c^≪N\hat c^\dagger \hat c \ll N, we see that

S^z=c^†c^−N2S^+=N c^†S−=N c^[c^,c^†]=1\hat S_z = \hat c^\dagger\hat c-\frac{N}{2}\qquad \hat S_+ = \sqrt{N}\,\hat c^\dagger \qquad S_- = \sqrt{N}\,\hat c\qquad [\hat c,\hat c^\dagger]=1

Clearly now the ensemble of atoms interacting with a single mode will be a perfectly bosonic wave.

Treat this as a fundamental structural change. Having cc fundamentally changes the structure of the algebra while retaining the known physical meaning. With cc, we are now able to use the single atom-photon interaction framework to treat the Dicke state ensemble.

Weak Excitation Regime§

The approximation c^†c^≪N\hat c^\dagger \hat c \ll N defines the weak excitation regime. In this regime, the collective spin behaves strictly as a harmonic oscillator. This justifies the use of linear optical tools, such as standard beam splitter relations, to fully describe the light-matter interface.

Beam splitter§

With this, the light-matter interaction with the ensemble can be written as

H^int=ℏ(geff a^c^†+geff∗ a^†c^)\hat H_\text{int} = \hbar (g_\text{eff}\,\hat a\hat c^\dagger + g_\text{eff}^*\,\hat a^\dagger \hat c)

Where geff=gNg_\text{eff} = g\sqrt{N}. This, is a beam splitter model.

Collective Rabi Oscillations and Quantum Memory§

Because the interaction takes the exact form of a beam splitter, the system undergoes collective Rabi oscillations between the photonic state ∣1⟩\ket{1} and the symmetric single-excitation Dicke state ∣S,m=−S+1⟩\ket{S, m=-S+1} at a frequency enhanced by N\sqrt{N}. This directly yields the famous vacuum Rabi splitting scaled by N\sqrt{N}.

Furthermore, this beam splitter interaction provides the natural framework for quantum memory. A single photon in the cavity mode can be completely mapped into the collective atomic excitation through a π\pi-pulse generated by this Hamiltonian.

Superradiance and Subradiance from Decay Rates§

Now that we have the beam splitter model and the exact expectation value ⟨S^+S^−⟩=ne(ng+1)\braket{\hat S^+\hat S^-}=n_e(n_g+1), calculating the collective decay rate is straightforward.

Assuming the atoms are confined to a volume much smaller than the wavelength (the standard Dicke limit so all atoms see the exact same radiation field), the total emission intensity of the ensemble is proportional to ⟨S^+S^−⟩\braket{\hat S^+\hat S^-}. If a single isolated atom decays at a rate Γ\Gamma, the total decay rate Γtot\Gamma_\text{tot} for a symmetric Dicke state ∣S,m⟩\ket{S,m} becomes:

Γtot=Γ⟨S^+S^−⟩=Γne(ng+1)\Gamma_\text{tot} = \Gamma \braket{\hat S^+\hat S^-} = \Gamma n_e(n_g+1)

To find the physical decay rate per excitation, we divide by the number of excited atoms nen_e:

Γper=Γne(ng+1)ne=Γ(ng+1)\Gamma_\text{per} = \frac{\Gamma n_e(n_g+1)}{n_e} = \Gamma (n_g+1)

Superradiance and the Superradiant Burst§

Let us look at the fully symmetric state with exactly a single excitation. Here, ne=1n_e = 1 and ng=N−1n_g = N-1. Plugging this into our formula gives Γper=ΓN\Gamma_\text{per} = \Gamma N, meaning the single excitation decays at a rate enhanced by a factor of NN compared to a single isolated atom.

Furthermore, consider the case where the ensemble is half excited such that ng=ne=N/2n_g = n_e = N/2. The total intensity becomes Γtot=ΓN2(N2+1)≈ΓN24\Gamma_\text{tot} = \Gamma \frac{N}{2}(\frac{N}{2} + 1) \approx \frac{\Gamma N^2}{4}. This demonstrates the characteristic N2N^2 intensity scaling of superradiance derived directly from the full coherent Dicke state expectation value.

As the system decays, ngn_g grows while nen_e shrinks. The per-excitation decay rate Γ(ng+1)\Gamma(n_g+1) increases as the atoms drop to the ground state. This positive feedback causes the emission to accelerate over time, concentrating the emitted energy into a short, intense pulse known as a superradiant burst.

Subradiance§

For symmetric Dicke states ∣S,m⟩\ket{S,m} with excitations, the ground state population is ng≥1n_g \ge 1, keeping the per-excitation decay rate proportional to Γ(ng+1)\Gamma (n_g+1). Subradiance corresponds to decay rates scaled below Γ\Gamma and arises from states with total spin S′<N/2S' < N/2. In these asymmetric states, the dipoles exhibit destructive interference. For example, with N=2N=2, the anti-symmetric singlet state 12(∣eg⟩−∣ge⟩)\frac{1}{\sqrt{2}}(\ket{eg} - \ket{ge}) has S′=0S'=0. This interference yields ⟨S^+S^−⟩=0\braket{\hat S^+\hat S^-} = 0 and a decay rate of zero.

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